Reconstruction of the time-dependent electronic wave packet arising from molecular autoionization

Roger Y. Bello; Sophie E. Canton; Denis Jelovina; John D. Bozek; Bruce Rude; Olga Smirnova; Mikhail Y. Ivanov; Alicia Palacios; Fernando Martín

doi:10.1126/sciadv.aat3962

Research ArticleChemistry

Reconstruction of the time-dependent electronic wave packet arising from molecular autoionization

Roger Y. Bello¹,
Sophie E. Canton²,³,
Denis Jelovina¹,
John D. Bozek⁴,
Bruce Rude⁵,
Olga Smirnova⁶,⁷,
Mikhail Y. Ivanov⁶,⁸,⁹,
Alicia Palacios ¹,¹⁰ and
Fernando Martín¹,¹¹,¹²,*

¹Departamento de Química, Módulo 13, Universidad Autónoma de Madrid, 28049 Madrid, Spain.
²Extreme Light Infrastructure Attosecond Light Pulse Source, ELI-HU Non-Profit Ltd., Dugonics ter 13, Szeged 6720, Hungary.
³Attosecond Science Group, Deutsches Elektronen-Synchrotron (DESY), Notkestrasse 85, D-22607 Hamburg, Germany.
⁴Synchrotron SOLEIL, L’Orme des Merisiers, Saint-Aubin, BP 48, 91192 Gif-sur-Yvette Cedex, France.
⁵Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA.
⁶Max-Born Institute for Nonlinear Optics and Short Pulse Spectroscopy, Max-Born-Straße 2A, D-12489 Berlin, Germany.
⁷Technische Universität Berlin, Ernst-Ruska-Gebäude, Hardenbergstr. 36 A, 10623 Berlin, Germany.
⁸Department of Physics, Imperial College London, South Kensington Campus, SW72AZ London, UK.
⁹Institute of Physics, Humboldt University Berlin, Newtonstrasse 15, 12489 Berlin, Germany.
¹⁰Institute for Advanced Research in Chemical Sciences, Universidad Autónoma de Madrid, 28049 Madrid, Spain.
¹¹Instituto Madrileño de Estudios Avanzados en Nanociencia, Cantoblanco, 28049 Madrid, Spain.
¹²Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, 28049 Madrid, Spain.

↵*Corresponding author. Email: fernando.martin{at}uam.es

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Science Advances 24 Aug 2018:
Vol. 4, no. 8, eaat3962
DOI: 10.1126/sciadv.aat3962

Roger Y. Bello

1Departamento de Química, Módulo 13, Universidad Autónoma de Madrid, 28049 Madrid, Spain.

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Sophie E. Canton

2Extreme Light Infrastructure Attosecond Light Pulse Source, ELI-HU Non-Profit Ltd., Dugonics ter 13, Szeged 6720, Hungary.

3Attosecond Science Group, Deutsches Elektronen-Synchrotron (DESY), Notkestrasse 85, D-22607 Hamburg, Germany.

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Denis Jelovina

1Departamento de Química, Módulo 13, Universidad Autónoma de Madrid, 28049 Madrid, Spain.

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John D. Bozek

4Synchrotron SOLEIL, L’Orme des Merisiers, Saint-Aubin, BP 48, 91192 Gif-sur-Yvette Cedex, France.

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Bruce Rude

5Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA.

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Olga Smirnova

6Max-Born Institute for Nonlinear Optics and Short Pulse Spectroscopy, Max-Born-Straße 2A, D-12489 Berlin, Germany.

7Technische Universität Berlin, Ernst-Ruska-Gebäude, Hardenbergstr. 36 A, 10623 Berlin, Germany.

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Mikhail Y. Ivanov

6Max-Born Institute for Nonlinear Optics and Short Pulse Spectroscopy, Max-Born-Straße 2A, D-12489 Berlin, Germany.

8Department of Physics, Imperial College London, South Kensington Campus, SW72AZ London, UK.

9Institute of Physics, Humboldt University Berlin, Newtonstrasse 15, 12489 Berlin, Germany.

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Alicia Palacios

1Departamento de Química, Módulo 13, Universidad Autónoma de Madrid, 28049 Madrid, Spain.

10Institute for Advanced Research in Chemical Sciences, Universidad Autónoma de Madrid, 28049 Madrid, Spain.

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Fernando Martín

1Departamento de Química, Módulo 13, Universidad Autónoma de Madrid, 28049 Madrid, Spain.

11Instituto Madrileño de Estudios Avanzados en Nanociencia, Cantoblanco, 28049 Madrid, Spain.

12Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, 28049 Madrid, Spain.

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For correspondence: fernando.martin@uam.es

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Reconstruction of the time-dependent electronic wave packet arising from molecular autoionization

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