Carbon-boron clathrates as a new class of sp3-bonded framework materials

Li Zhu; Gustav M. Borstad; Hanyu Liu; Piotr A. Guńka; Michael Guerette; Juli-Anna Dolyniuk; Yue Meng; Eran Greenberg; Vitali B. Prakapenka; Brian L. Chaloux; Albert Epshteyn; Ronald E. Cohen; Timothy A. Strobel

doi:10.1126/sciadv.aay8361

Research ArticleMATERIALS SCIENCE

Carbon-boron clathrates as a new class of sp³-bonded framework materials

View ORCID ProfileLi Zhu¹,
View ORCID ProfileGustav M. Borstad¹,*,
View ORCID ProfileHanyu Liu¹,†,
View ORCID ProfilePiotr A. Guńka¹,²,
View ORCID ProfileMichael Guerette¹,
View ORCID ProfileJuli-Anna Dolyniuk¹,
Yue Meng³,‡,
View ORCID ProfileEran Greenberg⁴,
View ORCID ProfileVitali B. Prakapenka⁴,
View ORCID ProfileBrian L. Chaloux⁵,
View ORCID ProfileAlbert Epshteyn⁵,
View ORCID ProfileRonald E. Cohen¹,⁶,⁷ and
View ORCID ProfileTimothy A. Strobel ¹,§

¹Geophysical Laboratory, Carnegie Institution for Science, 5251 Broad Branch Road, NW, Washington, DC 20015, USA.
²Faculty of Chemistry, Warsaw University of Technology, Noakowskiego 3, 00-664 Warszawa, Poland.
³High Pressure Collaborative Access Team, Geophysical Laboratory, Carnegie Institution for Science, Advanced Photon Source, Argonne, IL 60439, USA.
⁴Center for Advanced Radiation Sources, University of Chicago, Chicago, IL 60637, USA.
⁵Chemistry Division, U.S. Naval Research Laboratory, Washington, DC 20375, USA.
⁶Department of Earth and Environmental Sciences, Ludwig Maximilians Universität, Munich 80333, Germany.
⁷Department of Physics and Astronomy and London Centre for Nanotechnology, University College London, London, UK.

↵§Corresponding author. Email: tstrobel{at}carnegiescience.edu

↵* Present address: Department of Physics and Materials Science, University of Memphis, Memphis, TN 38152, USA.
↵† Present address: State Key Laboratory of Superhard Materials and Innovation Center for Computational Physics Methods and Software, College of Physics, Jilin University, Changchun 130012, China.
↵‡ Present address: HPCAT, X-ray Science Division, Argonne National Laboratory, Lemont, IL 60439, USA.

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Science Advances 10 Jan 2020:
Vol. 6, no. 2, eaay8361
DOI: 10.1126/sciadv.aay8361

Li Zhu

1Geophysical Laboratory, Carnegie Institution for Science, 5251 Broad Branch Road, NW, Washington, DC 20015, USA.

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Gustav M. Borstad

1Geophysical Laboratory, Carnegie Institution for Science, 5251 Broad Branch Road, NW, Washington, DC 20015, USA.

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Hanyu Liu

1Geophysical Laboratory, Carnegie Institution for Science, 5251 Broad Branch Road, NW, Washington, DC 20015, USA.

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Piotr A. Guńka

1Geophysical Laboratory, Carnegie Institution for Science, 5251 Broad Branch Road, NW, Washington, DC 20015, USA.

2Faculty of Chemistry, Warsaw University of Technology, Noakowskiego 3, 00-664 Warszawa, Poland.

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Michael Guerette

1Geophysical Laboratory, Carnegie Institution for Science, 5251 Broad Branch Road, NW, Washington, DC 20015, USA.

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Juli-Anna Dolyniuk

1Geophysical Laboratory, Carnegie Institution for Science, 5251 Broad Branch Road, NW, Washington, DC 20015, USA.

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Yue Meng

3High Pressure Collaborative Access Team, Geophysical Laboratory, Carnegie Institution for Science, Advanced Photon Source, Argonne, IL 60439, USA.

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Eran Greenberg

4Center for Advanced Radiation Sources, University of Chicago, Chicago, IL 60637, USA.

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Vitali B. Prakapenka

4Center for Advanced Radiation Sources, University of Chicago, Chicago, IL 60637, USA.

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Brian L. Chaloux

5Chemistry Division, U.S. Naval Research Laboratory, Washington, DC 20375, USA.

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Albert Epshteyn

5Chemistry Division, U.S. Naval Research Laboratory, Washington, DC 20375, USA.

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Ronald E. Cohen

1Geophysical Laboratory, Carnegie Institution for Science, 5251 Broad Branch Road, NW, Washington, DC 20015, USA.

6Department of Earth and Environmental Sciences, Ludwig Maximilians Universität, Munich 80333, Germany.

7Department of Physics and Astronomy and London Centre for Nanotechnology, University College London, London, UK.

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Timothy A. Strobel

1Geophysical Laboratory, Carnegie Institution for Science, 5251 Broad Branch Road, NW, Washington, DC 20015, USA.

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For correspondence: tstrobel@carnegiescience.edu

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