RT Journal Article SR Electronic T1 Dynamic fracture of tantalum under extreme tensile stress JF Science Advances JO Sci Adv FD American Association for the Advancement of Science SP e1602705 DO 10.1126/sciadv.1602705 VO 3 IS 6 A1 Albertazzi, Bruno A1 Ozaki, Norimasa A1 Zhakhovsky, Vasily A1 Faenov, Anatoly A1 Habara, Hideaki A1 Harmand, Marion A1 Hartley, Nicholas A1 Ilnitsky, Denis A1 Inogamov, Nail A1 Inubushi, Yuichi A1 Ishikawa, Tetsuya A1 Katayama, Tetsuo A1 Koyama, Takahisa A1 Koenig, Michel A1 Krygier, Andrew A1 Matsuoka, Takeshi A1 Matsuyama, Satoshi A1 McBride, Emma A1 Migdal, Kirill Petrovich A1 Morard, Guillaume A1 Ohashi, Haruhiko A1 Okuchi, Takuo A1 Pikuz, Tatiana A1 Purevjav, Narangoo A1 Sakata, Osami A1 Sano, Yasuhisa A1 Sato, Tomoko A1 Sekine, Toshimori A1 Seto, Yusuke A1 Takahashi, Kenjiro A1 Tanaka, Kazuo A1 Tange, Yoshinori A1 Togashi, Tadashi A1 Tono, Kensuke A1 Umeda, Yuhei A1 Vinci, Tommaso A1 Yabashi, Makina A1 Yabuuchi, Toshinori A1 Yamauchi, Kazuto A1 Yumoto, Hirokatsu A1 Kodama, Ryosuke YR 2017 UL http://advances.sciencemag.org/content/3/6/e1602705.abstract AB The understanding of fracture phenomena of a material at extremely high strain rates is a key issue for a wide variety of scientific research ranging from applied science and technological developments to fundamental science such as laser-matter interaction and geology. Despite its interest, its study relies on a fine multiscale description, in between the atomic scale and macroscopic processes, so far only achievable by large-scale atomic simulations. Direct ultrafast real-time monitoring of dynamic fracture (spallation) at the atomic lattice scale with picosecond time resolution was beyond the reach of experimental techniques. We show that the coupling between a high-power optical laser pump pulse and a femtosecond x-ray probe pulse generated by an x-ray free electron laser allows detection of the lattice dynamics in a tantalum foil at an ultrahigh strain rate of ~2 × 108 to 3.5 × 108 s−1. A maximal density drop of 8 to 10%, associated with the onset of spallation at a spall strength of ~17 GPa, was directly measured using x-ray diffraction. The experimental results of density evolution agree well with large-scale atomistic simulations of shock wave propagation and fracture of the sample. Our experimental technique opens a new pathway to the investigation of ultrahigh strain-rate phenomena in materials at the atomic scale, including high-speed crack dynamics and stress-induced solid-solid phase transitions.